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Thermophilic Pyrite Quorum Sensing Consortium

A moderately thermophilic three-species bioleaching consortium used to study the effects of quorum sensing (QS) signaling on pyrite and chalcopyrite dissolution. This acidophilic community consists of Leptospirillum ferriphilum DSM 14647, Acidithiobacillus caldus DSM 8584, and Sulfobacillus thermosulfidooxidans DSM 9293, operating at pH 2.0-2.5 and 40°C. The consortium demonstrates coordinated microbial behavior mediated by diffusible signal factor (DSF) and N-acyl-homoserine lactone (AHL) quorum sensing systems. Treatment with DSF-family compounds (DSF and BDSF at 2 μM each) reduced pyrite and chalcopyrite dissolution via inhibitory effects on iron oxidation and mineral colonization. DSF compounds induced A. caldus motility and dispersion from pyrite with concomitant expansion of L. ferriphilum on mineral surfaces, while AHL-mediated signaling (C12-AHL, C14-AHL, 3-OH-C12-AHL, 3-OH-C14-AHL at 5 μM each) repressed L. ferriphilum motility. The consortium was subjected to RNA-seq transcriptomics (12 samples, 271 Gbases) to elucidate gene expression changes in response to QS molecules (NCBI BioProject PRJNA1259591). This system represents the first comprehensive study of quorum sensing regulation in moderately thermophilic biomining bacteria, revealing that QS molecules change planktonic/mineral subpopulation distributions and modulate leaching efficiency through control of cell attachment and iron oxidation rates.

Taxonomy

Taxon Ontology ID Functional Roles Abundance
Leptospirillum ferriphilum NCBITaxon:178606
PRIMARY_PRODUCER PRIMARY_DEGRADER
DOMINANT
Acidithiobacillus caldus NCBITaxon:33059
PRIMARY_DEGRADER
ABUNDANT
Sulfobacillus thermosulfidooxidans NCBITaxon:28034
PRIMARY_PRODUCER PRIMARY_DEGRADER
ABUNDANT

Ecological Interactions

Ferrous Iron Oxidation by Leptospirillum

CROSS_FEEDING

Source Taxon: Leptospirillum ferriphilum

Metabolites: Fe(II) (CHEBI:29033), Fe(III) (CHEBI:29034)

Biological Processes:

Downstream Effects:
Pyrite and Chalcopyrite Dissolution

Evidence

  • doi:10.3389/fmicb.2025.1592588 - SUPPORT (IN_VIVO)
    "In addition, DSF compounds induced Acidithiobacillus caldus motility and dispersion from pyrite with a concomitant expansion of Leptospirillum ferriphilum on the mineral surface while in contrast, the acyl-homoserine lactone mediated QS system repressed L"
  • doi:10.3389/fmicb.2025.1592588 - SUPPORT (IN_VIVO)
    "DSF compounds induced concomitant expansion of Leptospirillum ferriphilum on the mineral surface"
  • doi:10.1038/s41598-021-95324-9 - SUPPORT (IN_VIVO)
    "Bioleaching of metal sulfide ores involves acidophilic microbes that catalyze the chemical dissolution of the metal sulfide bond that is enhanced by attached and planktonic cell mediated oxidation of iron(II)-ions and inorganic sulfur compounds"

Sulfur Oxidation by Acidithiobacillus caldus

MUTUALISM

Source Taxon: Acidithiobacillus caldus

Metabolites: sulfur (CHEBI:26833), sulfuric acid (CHEBI:26836)

Biological Processes:

Evidence

  • doi:10.3389/fmicb.2025.1592588 - SUPPORT (IN_VIVO)
    "In addition, DSF compounds induced Acidithiobacillus caldus motility and dispersion from pyrite with a concomitant expansion of Leptospirillum ferriphilum on the mineral surface while in contrast, the acyl-homoserine lactone mediated QS system repressed L"
  • doi:10.3389/fmicb.2025.1592588 - SUPPORT (IN_VIVO)
    "A decrease in mineral-attached populations of A. caldus was demonstrated after DSF addition"

Dual Iron and Sulfur Oxidation by Sulfobacillus

MUTUALISM

Source Taxon: Sulfobacillus thermosulfidooxidans

Metabolites: Fe(II) (CHEBI:29033), Fe(III) (CHEBI:29034), sulfur (CHEBI:26833), sulfuric acid (CHEBI:26836)

Biological Processes:

Evidence

  • doi:10.3389/fmicb.2025.1592588 - SUPPORT (IN_VIVO)
    "In this study, treatment of a moderately thermophilic biomining consortium with QS compounds, termed diffusible signal factors (DSF), reduced pyrite and chalcopyrite dissolution via an inhibitory effect on iron oxidation and mineral colonization by the mixed culture"
  • doi:10.3389/fmicb.2020.00044 - SUPPORT (IN_VITRO)
    "ferriphilum occurs during the dual-species biofilm formation, but different effects on bioleaching were noted, if the preculture of L"

Pyrite and Chalcopyrite Dissolution

MUTUALISM

Metabolites: pyrite (CHEBI:51905), chalcopyrite (CHEBI:50885), Fe(III) (CHEBI:29034), Fe(II) (CHEBI:29033), copper(2+) (CHEBI:29036), sulfuric acid (CHEBI:26836)

Biological Processes:

Downstream Effects:
Ferrous Iron Oxidation by Leptospirillum

Evidence

  • doi:10.3389/fmicb.2025.1592588 - SUPPORT (IN_VIVO)
    "In this study, treatment of a moderately thermophilic biomining consortium with QS compounds, termed diffusible signal factors (DSF), reduced pyrite and chalcopyrite dissolution via an inhibitory effect on iron oxidation and mineral colonization by the mixed culture"
  • doi:10.3389/fmicb.2025.1592588 - SUPPORT (IN_VIVO)
    "QS molecules change the planktonic/mineral subpopulations distribution of moderately thermophilic leaching bacteria"

DSF Quorum Sensing Signaling

MUTUALISM

Source Taxon: Leptospirillum ferriphilum

Metabolites: cis-11-methyl-2-dodecenoic acid (CHEBI:71190), (2Z)-2-dodecenoic acid (CHEBI:87659)

Biological Processes:

Evidence

  • doi:10.3389/fmicb.2025.1592588 - SUPPORT (IN_VIVO)
    "In this study, treatment of a moderately thermophilic biomining consortium with QS compounds, termed diffusible signal factors (DSF), reduced pyrite and chalcopyrite dissolution via an inhibitory effect on iron oxidation and mineral colonization by the mixed culture"
  • doi:10.3389/fmicb.2025.1592588 - SUPPORT (IN_VIVO)
    "treatment of a moderately thermophilic biomining consortium with QS compounds called diffusible signal factors (DSF) reduced pyrite and chalcopyrite dissolution"
  • doi:10.1038/s41598-021-95324-9 - SUPPORT (IN_VIVO)
    "In this study, we demonstrated a functional diffusible signal factor interspecies quorum sensing signaling mechanism in Leptospirillum ferriphilum and Leptospirillum ferrooxidans that produces (Z)-11-methyl-2-dodecenoic acid when grown with pyrite as energy source"

AHL Quorum Sensing Regulation

MUTUALISM

Source Taxon: Acidithiobacillus caldus

Metabolites: N-dodecanoyl-L-homoserine lactone (CHEBI:75314), N-tetradecanoyl-L-homoserine lactone (CHEBI:75315), N-(3-hydroxy-dodecanoyl)-L-homoserine lactone (CHEBI:75317), N-(3-hydroxy-tetradecanoyl)-L-homoserine lactone (CHEBI:75318)

Biological Processes:

Evidence

  • doi:10.3389/fmicb.2025.1592588 - SUPPORT (IN_VIVO)
    "In addition, DSF compounds induced Acidithiobacillus caldus motility and dispersion from pyrite with a concomitant expansion of Leptospirillum ferriphilum on the mineral surface while in contrast, the acyl-homoserine lactone mediated QS system repressed L"
  • doi:10.3389/fmicb.2025.1592588 - SUPPORT (IN_VIVO)
    "Some Acidithiobacillus species, including Acidithiobacillus caldus, possess a QS system mediated by acyl-homoserine lactones (AHLs)"

Environmental Factors

Factor Value Unit
Temperature 40 °C
pH 2.0-2.5 pH units
DSF Quorum Sensing Signals 2 μM
AHL Quorum Sensing Signals 5 μM
Mineral Substrates Pyrite and Chalcopyrite qualitative
RNA-Seq Transcriptomics 12 samples, 271 Gbases sequencing data
Oxygen Availability Aerobic qualitative